A General Approach to the Basiliolide/Transtaganolide Natural Products: Total Syntheses of Basiliolide B, epi‐8‐Basiliolide B, Transtaganolide C, and Transtaganolide D
Identifieur interne : 000051 ( Main/Exploration ); précédent : 000050; suivant : 000052A General Approach to the Basiliolide/Transtaganolide Natural Products: Total Syntheses of Basiliolide B, epi‐8‐Basiliolide B, Transtaganolide C, and Transtaganolide D
Auteurs : Hosea M. Nelson [États-Unis] ; Kei Murakami [États-Unis] ; Virgil [États-Unis] ; Stoltz [États-Unis]Source :
- Angewandte Chemie [ 0044-8249 ] ; 2011-04-11.
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Abstract
Blitzschnell: Die Totalsynthese von Transtaganolid‐ und Basiliolid‐Naturstoffen gelingt in drei Stufen ausgehend von achiralen monocyclischen Estern (siehe Schema). Entscheidende Schritte in der Synthese sind eine Ireland‐Claisen/Diels‐Alder‐Kaskade und eine neuartige Sequenz aus Methoxyacetylidkupplung und Cyclisierung.
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DOI: 10.1002/ange.201008003
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Nelson</name><affiliation wicri:level="2"><country xml:lang="fr">États-Unis</country><placeName><region type="state">Californie</region></placeName><wicri:cityArea>Warren and Katharine Schlinger Laboratory for Chemistry and Chemical Engineering, Division of Chemistry and Chemical Engineering, Caltech Center for Catalysis and Chemical Synthesis, California Institute of Technology, 1200 E. California Boulevard, MC 101‐20, Pasadena</wicri:cityArea></affiliation></author><author><name sortKey="Murakami, Kei" sort="Murakami, Kei" uniqKey="Murakami K" first="Kei" last="Murakami">Kei Murakami</name><affiliation wicri:level="2"><country xml:lang="fr">États-Unis</country><placeName><region type="state">Californie</region></placeName><wicri:cityArea>Warren and Katharine Schlinger Laboratory for Chemistry and Chemical Engineering, Division of Chemistry and Chemical Engineering, Caltech Center for Catalysis and Chemical Synthesis, California Institute of Technology, 1200 E. 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Chem.</title><idno type="ISSN">0044-8249</idno><idno type="eISSN">1521-3757</idno><imprint><publisher>WILEY‐VCH Verlag</publisher><pubPlace>Weinheim</pubPlace><date type="published" when="2011-04-11">2011-04-11</date><biblScope unit="volume">123</biblScope><biblScope unit="issue">16</biblScope><biblScope unit="page" from="3772">3772</biblScope><biblScope unit="page" to="3775">3775</biblScope></imprint><idno type="ISSN">0044-8249</idno></series><idno type="istex">300CF61072607D6271DCC18D3F72541C52BBAC16</idno><idno type="DOI">10.1002/ange.201008003</idno><idno type="ArticleID">ANGE201008003</idno></biblStruct></sourceDesc><seriesStmt><idno type="ISSN">0044-8249</idno></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Acetylide</term><term>Claisen‐Umlagerung</term><term>C‐C‐Kupplungen</term><term>Diels‐Alder‐Reaktion</term><term>Naturstoffsynthese</term></keywords></textClass><langUsage><language ident="en">en</language></langUsage></profileDesc></teiHeader><front><div type="abstract">Blitzschnell: Die Totalsynthese von Transtaganolid‐ und Basiliolid‐Naturstoffen gelingt in drei Stufen ausgehend von achiralen monocyclischen Estern (siehe Schema). Entscheidende Schritte in der Synthese sind eine Ireland‐Claisen/Diels‐Alder‐Kaskade und eine neuartige Sequenz aus Methoxyacetylidkupplung und Cyclisierung.</div></front></TEI><affiliations><list><country><li>États-Unis</li></country><region><li>Californie</li></region></list><tree><country name="États-Unis"><region name="Californie"><name sortKey="Nelson, Hosea M" sort="Nelson, Hosea M" uniqKey="Nelson H" first="Hosea M." last="Nelson">Hosea M. Nelson</name></region><name sortKey="Murakami, Kei" sort="Murakami, Kei" uniqKey="Murakami K" first="Kei" last="Murakami">Kei Murakami</name><name sortKey="Stoltz" sort="Stoltz" uniqKey="Stoltz" last="Stoltz">Stoltz</name><name sortKey="Virgil" sort="Virgil" uniqKey="Virgil" last="Virgil">Virgil</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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